Their visit to the academy, which is the home of the 1992 Cricket World Cup, won when Mr Khan captained the national team, saw the couple given bats for their three children, Prince George, Princess Charlotte and Prince Louis. The Duke and Duchess of Cambridge are in Pakistan as part of their Royal tour.
The Shaukat Khanum Memorial Cancer Hospital and Research Centre was started in the early 1990s by the cricket-hero-turned-politician Imran Khan, who is now Pakistan's prime minister, and whose first wife Jemima Goldsmith was a friend of the late princess.
Meanwhile, Prince William was a skilled player as he managed to get in six runs off of an excellent hit.
The Duchess of Cambridge added that she was "impressed" with her husband's geography knowledge.
While the Royal couple looked stunning in their traditional attires, it was the mode of transport they picked created quite a buzz on social media.
Prince William's mom visited the region on several occasions and even helped raise funds for a hospital in Pakistan that specializes in cancer treatments.
William and Kate's visit brought back memories for many Pakistanis who still love the late Lady Diana for her humanitarian work.
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William and Kate have travelled to Pakistan at the request of the Foreign and Commonwealth Office. Wafia Rehmani, 7, wore matching toy tiaras with Kate as she hosted a toy tea party on her bed.
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The Duke and Duchess of Cambridge also signed visitors book at the NCA. Kate and William's Pakistan visit will come to an end tomorrow.
Since arriving, the royal couple have been advocates for girls' education, visiting a girl's school in Islamabad.
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She prompt the viewers that they'd reminded her and William "precisely what family technique", sooner than finishing her address with some phrases in Urdu.
"The village we've seen here today is the best representation of that ideal that I could have possibly imagined", she said.
While it was all fun and games during the royals' cricket outing, they were spending time with children for an important cause: the British Council's DOSTI program.
Kensington Palace has called the Cambridges' five-day trip, which ends Friday, their "most complex" tour to date as the royals seek to boost ties between Britain and the second largest country in the Commonwealth. On her first visit in 1991, her trip to Lahore lasted only six hours during which she visited the Kinnaird College straight from the airport, followed by King Edward Medical College, the Millat Tractor Factory, Allama Iqbal mausoleum, Badshahi Mosque and Lahore Fort.