The death toll had stood at 72 on Saturday.
In Saharanpur district, the death toll climbed from 16 to 36, top administrative official Alok Pandey said.
The deaths occurred in the states of Uttar Pradesh and Uttarakhand.
Almost 100 people have died in Northern India after drinking tainted bootleg liquor. Authorities launched a crackdown and suspended police and officials.
In the adjoining Haridwar district, the death toll had risen to 28 from 12 on Friday, Indian broadcaster NDTV reported. "However, in the remaining cases unless the viscera report is not available, it is hard for doctors to ascertain clearly that the deaths were caused due to alcohol", A K Pandey, district magistrate Saharanpur said Saturday. Around 1,066 liters of hooch have been seized during the raid and over 50 people detained in state, reports said.
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In a neighbouring district a senior police officer said nine had died, adding that 66 suspected bootleggers had been arrested and samples of the liquor sent to a laboratory for testing.
They vowed to take strict action against the accused, saying they would demand death penalty for those involved in the illicit trade once the case reaches court.
The local governments in both the states have announced a compensation of 2,806 US dollars to the next of kin of each of those who died in the tragedy and 700 USA dollars for those taken ill.
Hundreds of poor people die every year in India due to alcohol poisoning, mostly from consuming cheap alcohol.
The liquor is usually made with poor-quality ingredients and sometimes mixed with industrial alcohol and toxic substances.